School of Physics (Journal Articles)

Permanent URI for this collectionhttps://hdl.handle.net/10539/38042

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    Kondo effect and enhanced magnetic properties in gadolinium functionalized carbon nanotube supramolecular complex
    (Nature Research, 2018-05) Ncube, S.; Coleman, C.; Strydom, A.; Flahaut, E.; de Sousa, A.
    We report on the enhancement of magnetic properties of multiwalled carbon nanotubes (MWNTs) functionalized with a gadolinium based supramolecular complex. By employing a newly developed synthesis technique, we find that the functionalization method of the nanocomposite enhances the strength of magnetic interaction, leading to a large effective moment of 15.79µB and nonsuperparamagnetic behavior, unlike what has been previously reported. Saturating resistance at low temperatures is ftted with the numerical renormalization group formula, verifying the Kondo effect for magnetic impurities on a metallic electron system. Magnetoresistance shows devices fabricated from aligned gadolinium functionalized MWNTs (Gd-Fctn-MWNTs) exhibit spin-valve switching behaviour of up to 8%. This study highlights the possibility of enhancing magnetic interactions in carbon systems through chemical modification, moreover, we demonstrate the rich physics that might be useful for developing spin based quantum computing elements based on one-dimensional (1D) channels.
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    Topological rejection of noise by quantum skyrmions
    (Nature Research, 2025-03) Ornelas, Pedro; Forbes, Andrew; de Mello Koch, Robert
    An open challenge in the context of quantum information processing and communication is improving the robustness of quantum information to environmental contributions of noise, a severe hindrance in real-world scenarios. Here, we show that quantum skyrmions and their nonlocal topological observables remain resilient to noise even as typical entanglement witnesses and measures of the state decay. This allows us to introduce the notion of digitization of quantum information based on our discrete topological quantum observables, foregoing the need for robustness of entanglement. We compliment our experiments with a full theoretical treatment that unlocks the quantum mechanisms behind the topological behavior, explaining why the topology leads to robustness. Our approach holds exciting promise for intrinsic quantum information resilience through topology, highly applicable to real-world systems such as global quantum networks and noisy quantum computers.
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    Entanglement beating in free space through spin–orbit coupling
    (Springer Nature, 2018) Rosales-Guzmán, Carmelo; Denz, Cornelia; Otte, Eileen; Ndagano, Bienvenu; Forbes, Andrew
    It is well known that the entanglement of a quantum state is invariant under local unitary transformations. This rule dictates, for example, that the entanglement of internal degrees of freedom of a photon remains invariant during free-space propagation. Here, we outline a scenario in which this paradigm does not hold. Using local Bell states engineered from classical vector vortex beams with non-separable degrees of freedom, the so-called classically entangled states, we demonstrate that the entanglement evolves during propagation, oscillating between maximally entangled (purely vector) and product states (purely scalar). We outline the spin–orbit interaction behind these novel propagation dynamics and confirm the results experimentally, demonstrating spin–orbit coupling in paraxial beams. This demonstration highlights a hitherto unnoticed property of classical entanglement and simultaneously offers a device for the on-demand delivery of vector states to targets, for example, for dynamic laser materials processing, switchable resolution within stimulated emission depletion (STED) systems, and a tractor beam for entanglement.